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You increased the enzyme concentration? Most Vmax values are given in "mol of product produced/s" so I'm not sure where the enzyme conc its in with that. I mean, obviously, you're going to be producing MORE moles of product/s with more enzyme but would it be correct to say that Vmax has increased? If you think about it, the Vmax for any particular enzyme is still the same (it still has the same efficiency)