As I understand it there are three paths to INR:
1. Radiology to Neuroradiology to INR
2. Neurosurgery to INR
3. Neurology to vascular neurology to INR
These are specified explicitly in the ACGME guidelines for endovascular surgical neuroradiology (i.e. INR), and all require 3+ months training in neurological examination, neuroradiology, and neurosurgery. The third path is difficult in the sense that there are only half a dozen programs that regularly take neurologists and another half a dozen that take them rarely. The first two paths are commonplace now.
Regarding which path is better: it depends partly on where you would like to practice. If you want to practice at a very large academic institution, option 1 will almost clearly train you best in the procedures themselves and allow you to have the support of other clinical specialties. If you want to practice INR privately, or at a much smaller institution, you will probably be best off with option 2 so that you can deal with the complications (unless you can find a neurosurgeon on call to take care of them for you... good luck!). I should note that path 3 is really designed for those who want to specialize in basic stroke INR procedures like IA thrombolysis and stenting so that complete stroke care can be delivered by a single physician. Path 3 INR folks are more akin to interventional cardiologist than interventional radiologists in the scope of their work.
In other words, if you want to be a maverick interventionalist at an academic institution and are sure about it, take option 1. If you want to work privately or are not sure about INR, take option 2 so that you can take the patient back if you need to or fall-back yourself on a different profession. If you want to be an 'interventional neurologist' for stroke patients, take option 3.
B